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A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the ${}^{229m}\mathrm{Th}$nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons and the number of ${}^{229m}\mathrm{Th}$embedded are determined for single crystalline ${\mathrm{CaF}}_2, {\mathrm{MgF}}_2, {\mathrm{LiSrAlF}}_6$, AlN, and amorphous ${\mathrm{SiO}}_2$. For the latter two materials, no radiative decay signal was observed and an upper limit of the ratio is reported. The radiative decay wavelength was determined in ${\mathrm{LiSrAlF}}_6$and ${\mathrm{CaF}}_2$, reducing its uncertainty by a factor of 2.5 relative to our previous measurement. This value is in agreement with the recently reported improved values from laser excitation. Published by the American Physical Society2025 

The cross-section of the thermal neutron capture⁴¹Ar(n,γ)⁴²Ar(t_1/2=32.9 y) reaction was measured by irradiating a⁴⁰Ar sample at the high-flux reactor of Institut Laue-Langevin (ILL) Grenoble, France. The signature of the two-neutron capture has been observed by measuring the growth curve and identifying the 1524.6 keV γ-lines of the shorter-lived⁴²K(12.4 h) β⁻daughter of⁴²Ar. Our preliminary value of the⁴¹Ar(n,γ)⁴²Ar thermal cross section is 240(80) mb at 25.3 meV. For the first time, direct counting of⁴²Ar was performed using the ultra-high sensitivity technique of noble gas accelerator mass spectrometry (NOGAMS) at Argonne National Laboratory, USA. 

The thermodynamical conditions and the neutron density produced in a laser-induced implosion of a deuterium-tritium (DT) filled capsule at the National Ignition Facility (NIF) are the closest laboratory analog of stellar conditions. We plan to investigate neutron-induced reactions on 40 Ar, namely the 40 Ar( n , 2 n ) 39 Ar( t 1/2 =268 y), the 40 Ar( n , γ) 41 Ar(110 min) and the potential rapid two-neutron capture reaction 40 Ar(2 n , γ) 42 Ar(33 y) in an Ar-loaded DT capsule. The chemical inertness of noble gas Ar enables reliable collection of the reaction products. 

Asymptotic giant branch stars are responsible for the production of most of the heavy isotopes beyond Sr observed in the solar system. Among them, isotopes shielded from the $r$-process contribution by their stable isobars are defined as $s$-only nuclei. For a long time the abundance of ${}^{204}\mathrm{Pb}$, the heaviest $s$-only isotope, has been a topic of debate because state-of-the-art stellar models appeared to systematically underestimate its solar abundance. Besides the impact of uncertainties from stellar models and galactic chemical evolution simulations, this discrepancy was further obscured by rather divergent theoretical estimates for the neutron capture cross section of its radioactive precursor in the neutron-capture flow, ${}^{204}\mathrm{Tl}$( $t_{1/2}=3.78\mathrm{yr}$), and by the lack of experimental data on this reaction. We present the first ever neutron capture measurement on ${}^{204}\mathrm{Tl}$, conducted at the CERN neutron time-of-flight facility n_TOF, employing a sample of only 9 mg of ${}^{204}\mathrm{Tl}$produced at the Institute Laue Langevin high flux reactor. By complementing our new results with semiempirical calculations we obtained, at the $s$-process temperatures of $kT\approx 8\mathrm{keV}$and $kT\approx 30\mathrm{keV}$, Maxwellian-averaged cross sections (MACS) of 580(168) mb and 260(90) mb, respectively. These figures are about 3% lower and 20% higher than the corresponding values widely used in astrophysical calculations, which were based only on theoretical calculations. By using the new ${}^{204}\mathrm{Tl}$MACS, the uncertainty arising from the ${}^{204}\mathrm{Tl}(\mathrm{n},\gamma )$cross section on the $s$-process abundance of ${}^{204}\mathrm{Pb}$has been reduced from $\sim 30\%$down to $+8\%/-6\%$, and the $s$-process calculations are in agreement with the latest solar system abundance of ${}^{204}\mathrm{Pb}$reported by K. Lodders in 2021. Published by the American Physical Society2024